Sains Malaysiana 52(1)(2023): 271-280

http://doi.org/10.17576/jsm-2023-5201-22

 

Penentuan Kepekatan Keradioaktifan Radionuklid Semula Jadi dan Indeks Bahaya Sinaran pada Musim Hujan dari Tanah di Kawasan Sekitar Kemudahan Simpanan Jangka Panjang (LTSF) Bukit Kledang, Perak

(Determination of Natural Radionuclide Radioactivity Concentration and Radiation Hazard Index during the Rainy Season from the Soil in the Area Around the Long-Term Storage Facility (LTSF) Bukit Kledang, Perak)

 

MOHD IZWAN ABDUL ADZIZ1 & KHOO KOK SIONG1,2,*

 

1Jabatan Fizik Gunaan, Fakulti Sains dan Teknologi, Universiti Kebangsaan Malaysia, 43600 UKM Bangi, Selangor Darul Ehsan, Malaysia

2Pusat Penyelidikan Teknologi (NUKLEAR), Fakulti Sains dan Teknologi, Universiti Kebangsaan Malaysia, 43600 UKM Bangi, Selangor Darul Ehsan, Malaysia

 

Recieved: 22 April 2022/Accepted: 30 September 2022

 

Abstrak

Kajian dan pemantauan yang dilakukan terhadap taburan dan penentuan aktiviti keradioaktifan radionuklid semula jadi boleh dijadikan panduan dan rujukan serta amat berguna terutamanya ketika berlakunya dedahan sinaran yang tinggi dan tidak terancang daripada sumber antropogenik dan kemalangan nuklear global. Sampel tanah permukaan dari 12 lokasi yang telah dikenal pasti di sekitar kawasan kemudahan repositori telah diambil untuk dijalankan kajian analisis penentuan kepekatan keradioaktifan dan indeks bahaya sinaran. Pengukuran kepekatan radioaktif dalam sampel tanah dilakukan dengan menggunakan sistem pembilangan spektrometer gama yang dilengkapi dengan pengesan High Purity Germanium (HPGe). Keputusan yang diperoleh menunjukkan kepekatan radioaktiviti 238U adalah berjulat antara 17.83 - 31.80 Bq kg-1, 234Th adalah berjulat antara 23.18 - 40.64 Bq kg-1, 226Ra adalah berjulat antara 20.09 - 32.80 Bq kg-1, 228Ra adalah berjulat antara 21.20 - 38.88 Bq kg-1 dan 40K adalah berjulat antara 9.11 - 51.39 Bq kg-1 dengan nilai purata masing-masing adalah 21.45 Bq kg-1, 28.17 Bq kg-1, 24.00 Bq kg-1, 27.43 Bq kg-1 dan 24.01 Bq kg-1. Nilai kepekatan radioaktiviti radionuklid tersebut didapati setara dengan nilai yang pernah dilaporkan dalam kajian terdahulu di Semenanjung Malaysia. Nilai purata yang diperoleh bagi keempat-empat parameter Indeks Bahaya Radiasi iaitu aktiviti bersamaan radium (Raeq), kadar dos luaran (D), dos berkesan tahunan dan indeks bahaya luaran (Hex) masing-masing adalah 66.37 Bq kg-1, 29.13 nGy j-1, 20.16 μSv dan 0.18. Nilai yang diperoleh ini adalah rendah berbanding nilai purata dunia dan nilai piawaian yang diguna pakai secara global iaitu masing-masing adalah 370 Bq kg-1, 57nGy j-1, 480.00 μSv dan 1.0. Perbandingan dengan kajian sebelum ini juga mendapati nilai bagi keempat-empat parameter adalah rendah dan setara. Ini menunjukkan tahap bahaya radiasi di kawasan sekitar kajian adalah selamat untuk orang ramai.

 

Kata kunci: Bahan radioaktif semula jadi; kemudahan repositori; musim hujan; spektrometer gama; tanah

 

Abstract

Continuous research and monitoring on the distribution and determination of these natural radionuclides' activity as a guide and reference and are very useful, especially in an accidental exposure. Surface soil samples from 12 locations that have been identified around the repository facility area were taken for the study. Radioactive concentrations in soil samples were measured using a gamma spectrometer counting system equipped with an HPGe detector. The results obtained showed that the radioactivity concentration of 238U ranged between 17.83 - 31.80 Bq kg-1, 234Th ranged between 23.18 - 40.64 Bq kg-1, 226Ra ranged between 20.09 - 32.80 Bq kg-1, 228Ra ranged between 21.20 - 38.88 Bq kg-1 and 40K ranged between 9.11-51.39 Bq kg-1 with average values ​​of 21.45 Bq kg-1, 28.17 Bq kg-1, 24.00 Bq kg-1, 27.43 Bq kg-1, and 24.01 Bq kg-1, respectively. The values obtained from this study were low or equivalent to the values previously reported in previous studies. It was also found that the mean/mean values obtained for the four parameters of the Radiation Hazard Index, namely radium equivalent activity (Raeq), external dose rate (D), annual effective dose and external hazard index (Hex) were 66.37 Bq kg-1, 29.13 nGy h-1, 20.16 μSv and 0.18, respectively. These obtained values are low compared to the world average values and the values of globally applied standards (370 Bq kg-1, 57nGy h-1, 480.00 μSv & 1.0, respectively). Comparison with previous studies also found that the values for all four parameters were low and equivalent. This indicates that the level of radiation hazard in the area around the study is safe for the public.

 

Keywords: Gamma spectrometer; natural radioactive material; soil; repository facility; wet season

 

REFERENCES

Adziz, M.I.A. & Khoo, K.S. 2018. An assessment of absorbed dose and radiation hazard index from soil around repository facility at Bukit Kledang, Perak, Malaysia. IOP Conf. Ser.: Mater. Sci. Eng. 298: 01200.

Al-Kaabi, M.A. & Al-Shimary, A. 2016. Study of the radiological doses and hazard indices in soil samples from Karbala City, Iraq. Chines Physics 16: 331-347.

Almayahi, B.A., Tajuddin, A.A. & Jaafar, M.S. 2012. Radiation hazard indices of soil and water samples in northern Malaysian Peninsular. International Journal of Applied Radiation and Isotopes 70(11): 2652-2660.

Anagnostakis, M.J., Hinis, E.P., Simopoulos, S.E. & Angelopoulos, M.G. 1996. Natural radioactivity mapping of greek surface soils. Environmental International 22(1): 3-8.

Dovlete, C. & Povinec, P.P. 2002. Quantification of uncertainty in gamma spectrometric analysis of environmental samples. 2nd Regional Training Course on QA/QC of Nuclear Analytical Techniques, 12-16 August. Kuala Lumpur.

Hemby, D.M. & Tynybekov, A.K. 2012. Uranium, thorium and potassium in soils along the shore of the lake Issyk-Kyol in the Kyrghyz Republic. Environ. Monit. Assess 73: 101-108.

Hussain, A. 1994. Deterpurataation of uranium and thorium concentration in rock samples. J. Radioanal. Nucl. Chem. 188(4): 255-265.

Iqbal, M., Tufail, M. & Mirza, S.M. 2000. Measurement of natural radioactivity in marble found in Pakistan using a NaI(Tl) gamma-ray spectrometer. Journal of Environmental Radioactivity 51(2): 255-265.

Krieger, R. 1981. Radioactivity of construction materials. Betonwerk und Fertigteil-Technik/Concrete Precasting Plant and Technology 47: 468.

Lee, S.K., Husin, W., Ahmad Termizi, R. & Nursama, H.A. 2007. Natural gamma background radiation dose rate and its relationship with geological background in the Kinta district, Perak, Malaysia. Applied Radiation and Isotopes 54: 327-333.

OECD. 1998. Uranium 1997 - Resources, Production and Demand. Paris: OECD.

Ogundele, K.T., Oluyemi, E.A., Oyekunle, J.A.O., Makinde, O.W. & Gbenu, S.T. 2018. An evaluation of health hazards indices of natural radioactivity of the sediments from Eko-Ende Dam, Osun State, Nigeria. Open Journal of Ecology 8: 607-621. https://doi.org/10.4236/oje.2018.811036

Saffuwan Mohamed Johar, Saiful Azhar Ahmad Tajudin & Zaidi Embong. 2016. The gamma dose assessment and pH correlation for various soil types at Batu Pahat and Kluang districts, Johor. AIP Conference Proceedings 1704: 050007. https://doi.org/10.1063/1.4940103

Shender, M.A. 1997. Measurement of natural radioactivity levels in soil in Tripoli. Applied Radiation and Isotopes 48(1): 147-148.

Tzortzis, M., Svoukis, E. & Tsetos, H. 2004. A comprehensive study of natural gamma radioactivity levels and associated dose rates from surface soils in Cyprus. Radiation Protection Dosimetry 109(3): 217-224.

UNSCEAR. 2000. Radiation Sources and Effects of Ionizing Radiation. New York: United Nations Scientific Committee on the Effect of Atomic Radiation.

UNSCEAR. 1982. Ionizing Radiation: Sources and Biological Effects. New York: United Nations.

Yang, Y.X., Wu, X.M., Jiang, Z.Y., Wang, W.X., Lu, J.G., Lin, J., Wang, L.M. & Hsia, Y.F. 2005. Radioactivity concentrations in soils of the Xiazhuang granite area, China. Appl. Radiat. Isot. 63: 255-259.

Yasir, M.S., Majid, A.A., Tap, M.S.Q. & Abidin, M.R.Z. 2006. Analisis 238U, 232Th, 226Ra dan 40K dalam sampel amang, tanah dan air di Dengkil, Selangor menggunakan spektometri sinar gama. Malaysia Journal of Analytical Sciences 10(1): 35-40.

Zal U’yun, W.M., Yii, M.W., Mohd Ashhar, K., Khairuddin, M.K., Abdul Kadir, I. & Mohd Abd Wahab, Y. 2017. Assessment of natural radioactivity level and radiological index in the vicinity of lynas rare-earth processing plants. ASEAN J. Sci. Technol. Dev. 34(2): 67-78.

 

*Corresponding author; email: khoo@ukm.edu.my

 

 

 

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